恒流通截面旋轉(zhuǎn)填充床流體流動(dòng)與傳質(zhì)性能研究

恒流通截面旋轉(zhuǎn)填充床流體流動(dòng)與傳質(zhì)性能研究摘要

針對(duì)恒流通截面旋轉(zhuǎn)填充床在流體流動(dòng)與傳質(zhì)性能方面的研究，本文以計(jì)算流體力學(xué)理論為基礎(chǔ)，采用數(shù)值模擬方法對(duì)旋轉(zhuǎn)填充床內(nèi)部流動(dòng)及傳質(zhì)進(jìn)行了探究。

通過對(duì)實(shí)驗(yàn)室內(nèi)構(gòu)造的實(shí)物旋轉(zhuǎn)填充床進(jìn)行CFD數(shù)值模擬，對(duì)床層內(nèi)部流動(dòng)進(jìn)行了展開研究，得到了填充床內(nèi)部速度場(chǎng)、壓力場(chǎng)、濃度場(chǎng)的變化規(guī)律。基于小波分析，還運(yùn)用時(shí)間尺度分析方法研究了床層流動(dòng)的脈動(dòng)特性。通過模擬結(jié)果可以發(fā)現(xiàn)，旋轉(zhuǎn)填充床床層內(nèi)部流動(dòng)存在著強(qiáng)烈的脈動(dòng)性和旋轉(zhuǎn)性，流動(dòng)狀態(tài)在流通截面上呈現(xiàn)出不均勻分布的特點(diǎn)，其中夾層流動(dòng)和渦流運(yùn)動(dòng)是較為明顯的兩種流動(dòng)形式。

同時(shí)，本文還對(duì)床層內(nèi)部傳質(zhì)情況進(jìn)行了研究和分析，得出了旋轉(zhuǎn)填充床的質(zhì)量傳遞效率和床層內(nèi)部傳質(zhì)效應(yīng)特點(diǎn)。在質(zhì)量傳遞效率研究方面，本文還探討了床層內(nèi)填充物密度、液體物性和旋轉(zhuǎn)速度等因素對(duì)床層內(nèi)傳質(zhì)效率的影響，并且運(yùn)用機(jī)器學(xué)習(xí)方法建立了傳質(zhì)效率預(yù)測(cè)模型。

關(guān)鍵詞：旋轉(zhuǎn)填充床；CFD數(shù)值模擬；傳質(zhì)效率；夾層流動(dòng)；機(jī)器學(xué)習(xí)。

Abstract

Thisstudyinvestigatesthefluidflowandmasstransferperformanceoftheconstantcross-sectionrotatingpackedbedbyusingcomputationalfluiddynamics(CFD)simulations.

Theflowcharacteristicsofthepackedbed,includingvelocity,pressure,andconcentrationfields,wereanalyzedthroughnumericalsimulationsofthephysicalrotatingpackedbedconstructedinthelaboratory.Time-scaleanalysisbasedonwaveletanalysiswasusedtoinvestigatethepulsatingcharacteristicsoftheflowinthebed.Thesimulationresultsshowthattheflowinthepackedbedischaracterizedbystrongpulsatingandrotatingflowsandexhibitsanon-uniformdistributioninthecross-sectionalarea.Twoflowpatterns,interlayerflowandvortexflow,areevident.

Inaddition,themasstransfercharacteristicsofthepackedbedwerealsoanalyzed,andthemasstransferefficiencyandinternalmasstransfereffectswerestudied.Thispaperalsoinvestigatedtheeffectsofpackingdensity,fluidproperties,androtationalspeedonthemasstransferefficiencyinthepackedbedandestablishedapredictionmodelforthemasstransferefficiencyusingmachinelearningalgorithms.

Keywords:rotatingpackedbed;CFDsimulation;masstransferefficiency;interlayerflow;machinelearning.TheresultsoftheCFDsimulationsshowedthattheinterlayerflowplaysanimportantroleinthemasstransferefficiencyintherotatingpackedbed.Theinterlayerflowcansignificantlyenhancethemasstransferefficiencyandreducetheinternalmasstransfereffects.Theanalysisofthefluidflowcharacteristicsrevealedthattheinterlayerflowismainlydrivenbythecentrifugalforcesandthedensitydifferencesbetweenthefluidlayers.

Thepackingdensitywasfoundtohaveasignificanteffectonthemasstransferefficiencyinthepackedbed.Themasstransferefficiencyincreasedwiththepackingdensity,asthehigherdensityresultsinahigherinterlayerflowandmoreeffectivecontactbetweenthefluidphases.Thefluidproperties,suchasviscosityandsurfacetension,alsohadaninfluenceonthemasstransferefficiency.Higherviscosityandsurfacetensionwerefoundtoreducetheinterlayerflowandincreasetheinternalmasstransfereffects.

Therotationalspeedofthepackedbedwasfoundtohaveanonlineareffectonthemasstransferefficiency.Atlowrotationalspeeds,theinterlayerflowandmasstransferefficiencyincreasedwiththerotationalspeed.However,athighrotationalspeeds,theinterlayerflowwashinderedbythecentrifugalforcesandthemasstransferefficiencydecreased.Apredictionmodelforthemasstransferefficiencywasestablishedbasedonmachinelearningalgorithms,whichcanbeusedtooptimizethedesignandoperationoftherotatingpackedbed.

Insummary,theCFDsimulationsandanalysisoftheflowcharacteristicsandmasstransferefficiencyinarotatingpackedbedprovidevaluableinsightsintotheoperationandoptimizationofthistechnology.Theresultscanbeusedtoguidethedesignandscale-upofrotatingpackedbedsforvariousapplicationsinchemicalengineeringandbiotechnology.Furthermore,theuseofexperimentalvalidationdatacanenhancetheaccuracyoftheCFDsimulations,andaidinthedevelopmentofmorepreciseandreliablemodels.Additionally,theincorporationofmachinelearningalgorithmscanprovideapowerfultoolforoptimizingthedesignandoperationofrotatingpackedbeds,enablingengineersandresearcherstorapidlyidentifytheoptimalparametersfortheirspecificapplication.

Moreover,theapplicationofrotatingpackedbedsisnotlimitedtochemicalengineeringandbiotechnology,butalsohaspotentialapplicationsinawiderangeofindustries,suchasenergy,foodprocessing,andenvironmentalremediation.Forexample,rotatingpackedbedscanbeusedfortheseparationofcarbondioxidefromfluegasinpowerplants,orforthepurificationofwastewaterinmunicipaltreatmentfacilities.

Inconclusion,theanalysisoftheflowcharacteristicsandmasstransferefficiencyinarotatingpackedbedusingCFDsimulationsprovidesimportantinsightsintothedesignandoperationofthistechnology.Bycombiningexperimentalvalidationandmachinelearningalgorithms,engineersandresearcherscandevelopmoreaccurateandprecisemodels,andoptimizetherotatingpackedbedforvariousapplicationsindifferentindustries.Thepotentialbenefitsofthistechnologyaresignificant,anditsusecanleadtomoreefficientandsustainableprocesses,aswellasprovideacost-effectivesolutionforavarietyofseparationandpurificationchallenges.Apartfromtheareaswhererotatingpackedbedshavealreadybeenused,thereareseveralotherindustrieswherethistechnologycanbeapplied.Forinstance,inthepharmaceuticalindustry,thesebedscanbeusedtoseparatechiralcompounds,whicharemirrorimagesofeachotherandhavedifferentpharmacologicalproperties.Byusingrotatingpackedbeds,itispossibletoachievehighchiralpurityandenantiomericexcessofthedesiredcompound,whichcanleadtothedevelopmentofmoreeffectivetherapeuticproducts.

Similarly,inthefoodandbeverageindustry,rotatingpackedbedscanbeusedtoextractbioactivecompoundsfromnaturalsourcessuchasfruits,vegetables,andherbs.Thesecompounds,suchaspolyphenols,carotenoids,andflavonoids,havenumeroushealthbenefitsandareoftenusedasingredientsinfunctionalfoodanddietarysupplements.Byusingrotatingpackedbeds,itispossibletoextractthesecompoundsinamoreefficientandenvironmentallyfriendlywaycomparedtotraditionalextractionmethodssuchassolventextractionorsupercriticalfluidextraction.

Anotherpotentialapplicationofrotatingpackedbedsisinthechemicalindustry,particularlyintheproductionoffinechemicalsandspecialtychemicals.Forexample,rotatingpackedbedscanbeusedtoseparateandpurifycomplexmixturesofchemicals,includingisomers,stereoisomers,anddifferenthomologues.Byoptimizingtheoperatingparametersofthebed,itispossibletoachievehighpurityandyieldofthedesiredproduct,whichcanreducetheoverallproductioncostsandincreasetheprofitabilityoftheprocess.

Inconclusion,rotatingpackedbedsareapromisingtechnologyforvariousseparationandpurificationchallengesindifferentindustries.Thecombinationofexperimentalvalidationandmachinelearningalgorithmscanleadtothedevelopmentofmoreaccurateandprecisemodels,whichcanoptimizetheperformanceofthebedandimproveitsefficiencyandsustainability.Withfurtherresearchanddevelopment,rotatingpackedbedshavethepotentialtobecomeacost-effectiveandenvironmentallyfriendlysolutiontomanyseparationandpurificationproblems.Inadditiontotheirapplicationsinseparationandpurificationprocesses,rotatingpackedbedsalsohavepotentialforuseinotherindustries.Forexample,thetechnologycouldbeappliedinthefoodindustryforthedehydrationoffruitsandvegetables,aswellastheproductionofconcentratedjuicesandsauces.Itcouldalsobeusefulinwastewatertreatmentprocesses,particularlyfortheseparationandremovalofpollutantsfromwatersources.

Anotherpotentialapplicationofrotatingpackedbedsisinthefieldofenergyproduction.Thetechnologycouldbeusedtoseparateandpurifydifferentgasesintheproductionoffuel,suchasthepurificationofhydrogenforuseinfuelcells.Itcouldalsobeusefulincarboncaptureandsequestrationprocesses,whichaimtoreducecarbonemissionsfrompowerplantsandothersources.

However,furtherresearchisneededtooptimizethedesignandoperationofrotatingpackedbedsforthesevariousapplications.Advancesincomputationalmodelingandsimulationwillbeparticularlyimportantforunderstandingtheunderlyingphysicsoffluidflowandmasstransferinthesesystems.Improvedunderstandingofthesecomplexitieswillenableresearcherstodevelopmoreaccurateandpredictivemodelsthatcanbeusedtooptimizetheperformanceofrotatingpackedbedsindifferentindustrialsettings.

Overall,rotatingpackedbedsrepresentapromisingtechnologyforseparatingandpurifyingfluidsinavarietyofindustrialsettings.Withcontinuedresearchanddevelopment,thistechnologyhasthepotentialtoimprovetheefficiencyandsustainabilityofmanyindustrialprocesses,whilealsoreducingtheirenvironmentalimpact.Oneofthekeyadvantagesofrotatingpackedbedsistheirabilitytoperformcomplexseparationswithhigherefficiencyandlowerenergyconsumptioncomparedtoconventionalseparationmethods.Forexample,inthepetrochemicalindustry,rotatingpackedbedscanbeusedfortheseparationofdifferenthydrocarbonsincrudeoil,aswellasforthepurificationofnaturalgasandothergases.Inthepharmaceuticalindustry,rotatingpackedbedsareusedfortheseparationandpurificationofvariousdrugs,aswellasforproteinfractionationandrecovery.

Anotherpotentialapplicationofrotatingpackedbedsisinthetreatmentofwastewaterandotherindustrialeffluents.Dependingonthespecificcontaminantspresentinthewastewater,rotatingpackedbedscanbedesignedtotargetandselectivelyremovethosecontaminants,suchasheavymetals,organicpollutants,andmicroorganisms.Inadditiontoimprovingthequalityofthetreatedwater,thiscanalsoreducetheamountoftoxicwastethatneedstobedisposedof,therebyreducingtheenvironmentalimpactofindustrialoperations.

Despitetheirmanyadvantages,therearestillsomechallengesassociatedwiththeuseofrotatingpackedbedsthatneedtobeaddressedinfutureresearch.Forexample,thereisaneedtoimprovetheunderstandingofthephysicalandchemicalprocessesthatoccurwithintherotatingpackedbed,inordertooptimizetheperformanceandminimizetheenergyconsumption.Additionally,therearestillsomelimitationsinthematerialsusedforthepacking,whichcanbepronetofouling,corrosion,andotherformsofdegradationovertime.

Nevertheless,withcontinuedresearchanddevelopment,itislikelythatrotatingpackedbedswillbecomeanincreasinglyimportanttechnologyforawiderangeofindustrialapplications.Byprovidingmorepreciseandefficientseparationandpurification,thistechnologyhasthepotentialtoimprovethesustainabilityandenvironmentalimpactofmanydifferentindustries,whilealsoreducingthecostsassociatedwithwastedisposalandenergyconsumption.Asrotatingpackedbedscontinuetoberesearchedanddeveloped,potentialapplicationsarebeingidentifiedinadiverserangeofindustries.Oneareaofinterestisinthetreatmentofindustrialwastewater.Manydifferenttypesofindustrialprocessesproducewastewaterthatmustbetreatedbeforeitcanbedischargedintotheenvironment.Conventionaltreatmentmethodssuchassedimentationandfiltrationcanbeslowandinefficient,resultinginhighoperatingcostsandasignificantenvironmentalfootprint.

Rotatingpackedbeds,ontheotherhand,offeralow-maintenanceandenergy-efficientalternativeforthetreatmentofindustrialwastewater.Byprovidingahighsurfaceareaformasstransfer,thesesystemsarecapableofremovingcontaminantssuchasheavymetals,organiccompounds,andsuspendedsolidsatafasterratethantraditionaltreatmentmethods.Additionally,thecompactsizeofthesesystemsmeanstheycanbeeasilyintegratedintoexistingtreatmentplants,reducingtheneedforexpensiveupgradesorretrofitting.

Anotherpotentialapplicationforrotatingpackedbedsisintheproductionofbiofuels.Asdemandsforrenewableenergysourcescontinuetogrow,biofuelsarebecominganincreasinglyimportantpartoftheenergymix.However,theproductionofbiofuelsfrombiomasscanbeenergy-intensiveandcostlyduetotheneedforcomplexseparationandpurificationprocesses.Rotatingpackedbedsofferapotentialsolutiontothischallengebyprovidingamoreefficientandcost-effectivewaytoseparateandpurifybiofuelsfromthebiomass.

Inadditiontowastewatertreatmentandbiofuelproduction,rotatingpackedbedsalsohavepotentialapplicationsinthepharmaceuticalindustry.Onecriticalstepinpharm